滴滴涕类农药在广东省鱼类中的残留及人体暴露水平初步评价DDT Residues in Typical Fishes of Guangdong Province and Human Exposure via Fish Consumption
孟祥周;余莉萍;郭英;郭建阳;罗孝俊;麦碧娴;曾永平;
摘要(Abstract)：
检测了采自广东省13个城市水产市场和超市的390个鱼样品中滴滴涕类农药(DDT)及其代谢物(包括o,p’-DDE,p,p’-DDE,o,p’-DDD,p,p’-DDD,o,p’-DDT,p,p’-DDT)的残留浓度.鱼体中DDTs的含量为8.7￣18002ng·g-1(脂肪重)或0.1￣698.9ng·g-1(湿重).不同鱼类之间因生活环境和生活习性的不同,而使其DDTs含量存在较大差别.与我国鱼类食品中DDTs的残留标准相比,仅有2个样品中的DDTs含量水平超过此标准,约占样品总数的0.51%,而超过欧盟水产品标准和美国环境保护局(EPA)标准的样品分别占13.8%和30.5%.广东省居民通过鱼类消费每天DDTs的摄入量为30.8ng·kgbodyweight-1·day-1,仅占FAO/WHO每日允许摄入量的0.3%,但高于其他国家或地区.
关键词(KeyWords)： 滴滴涕;鱼类;人体暴露;广东省
基金项目(Foundation): 国家自然科学基金(No.40532013);; 中国科学院“引进国外杰出人才计划”基金
作者(Author): 孟祥周;余莉萍;郭英;郭建阳;罗孝俊;麦碧娴;曾永平;
Email:
DOI:
参考文献(References)：
- AmatoCD,TorresJP,MalmO,BastosW,ClaudioL,MarkowitzS.2004.DDTinfishesfromfourdifferentAmazonsites:exposureassessmentforbreastfeedinginfants[J].OrganohalogenCompounds,66:2483-2490
- AnTC,ChenJX,FuJM,ShengGY,LiGY,HuZY,KuangYQ.2005.ThepollutionsituationandcontrolstrategyofpersistentorganicpollutantsinthePearlRiverDelta,China[J].EcologyandEnvrionment,14(6):981-986(inChinese)
- BinelliA,ProviniA.2003.POPsinedibleclamsfromdifferentItalianandEuropeanmarketsandpossiblehumanhealthrisk[J].MarPollutBull,46(7):879-886
- ErdogrulO,CovaciA,SchepensP.2005.Levelsoforganochlorinepesticides,polychlorinatedbiphenylsandpolybrominateddiphenylethersinfishspeciesfromKahramanmaras,Turkey[J].EnvironInt,31(5):703-711
- KipcicD,VukusicJ,SebecicB.2002.MonitoringofchlorinatedhydrocarbonpollutionofmeatandfishinCroatia[J].FoodTechnolBiotechnol,40(1):39-47
- KongKY,CheungKC,WongCK,WongMH.2005.TheresidualdynamicofpolycyclicaromatichydrocarbonsandorganochlorinepesticidesinfishpondsofthePearlRiverdelta,SouthChina[J].WaterRes,39(9):1831-1843
- KumbladL,OlssonA,KoutnyV,BergH.2001.DistributionofDDTresiduesinfishfromtheSongkhlaLake,Thailand[J].EnvironPollut,112(2):193-200
- LiWH,ZhangYH,FanQY,NakataH,KitanoT,AbeS,DingXC.2005.Currentstatusoforganchlorinepesticidescontaminationinfoodstuffsandhumanbreastfattissues[J].JEnvironOccupMed,22(1):14-16(inChinese)
- LiangCH,DengF,HuangWX,LiH,ChenM,LiuZW,LiangXX,LiangFR,CaiWH,LiangHJ.2003.NetworkmonitoringanddynamicanalysisofchemicalcontaminantsinagriculturalproductsinGuangdong[J].ChineseJournaloffoodhygiene,15(5):395-400(inChinese)
- LuoX,MaiB,YangQ,FuJ,ShengG,WangZ.2004.Polycyclicaromatichydrocarbons(PAHs)andorganochlorinepesticidesinwatercolumnsfromthePearlRiverandtheMacaoharborinthePearlRiverDeltainSouthChina[J].MarPollutBull,48(11-12):1102-1115
- LuoXJ,ChenSJ,MaiBX,ZengEY.2006.Source,transportandriskassessmentofPAHsinsurfacesedimentsfromPearlRiverDelta[J].AsianJournalofEcotoxicology,1(1):17-24(inChinese)
- ManirakizaP,CovaciA,NizigiymanaL,NtakimaziG,SchepensP.2002.PersistentchlorinatedpesticidesandpolychlorinatedbiphenylsinselectedfishspeciesfromLakeTanganyika,Burundi,Africa[J].EnvironPollut,117(3):447-455
- MonirithI,UenoD,TakahashiS,NakataH,SudaryantoA,SubramanianA,KaruppiahS,IsmailA,MuchtarM,ZhengJ,RichardsonBJ,PrudenteM,HueND,TanaTS,TkalinAV,TanabeS.2003.Asia-Pacificmusselwatch:monitoringcontaminationofpersistentorganochlorinecompoundsincoastalwatersofAsiancountries[J].MarPollutBull,46(3):281-300
- NakataH,KawazoeM,ArizonoK,AbeS,KitanoT,ShimadaH,LiW,DingX.2002.Organochlorinepesticidesandpolychlorinatedbiphenylresiduesinfoodstuffsandhumantissuesfromchina:statusofcontamination,historicaltrend,andhumandietaryexposure[J].ArchEnvironContamToxicol,43(4):473-480
- NakataH,NasuT,AbeS,KitanoT,FanQ,LiW,DingX.2005.OrganochlorinecontaminantsinhumanadiposetissuesfromChina:massbalanceapproachforestimatinghistoricalChineseexposuretoDDTs[J].EnvironSciTechnol,39(13):4714-4720
- SankarTV,ZynudheenAA,AnandanR,ViswanathanNairPG.2006.DistributionoforganochlorinepesticidesandheavymetalresiduesinfishandshellfishfromCalicutregion,Kerala,India[J].Chemosphere,(inpress)
- SunF,WongSS,LiGC,ChenSN.2006.Apreliminaryassessmentofconsumer’sexposuretopesticideresiduesinfisheriesproducts[J].Chemosphere,62(4):674-680
- WangMQ,WangZT,RanL,HanHW,WangYF,YangDJ.2002.StudyonfoodcontaminantsmonitoringinChinaduring2000-2001[J].JournalofHygieneResearch,32(4):322-326(inChinese)
- WongMH,LeungAO,ChanJK,ChoiMP.2005.AreviewontheusageofPOPpesticidesinChina,withemphasisonDDTloadingsinhumanmilk[J].Chemosphere,60(6):740-752
- WuXS.2006.TheregionalcompetitionanalysisandthefuturedevelopingstrategyofChinesefishery[OL].2006.5.10,http://www.chinafeed.org.cn/cms/_code/business/include/php/180687.htminChinese)
- YangN,Matsu1daM,KawanoM,WakimotoT.2005.PCBsandorganochlorinepesticides(OCPs)inediblefishandshellfishfromChina[J].Chemosphere,(inpress)
- YehouenouAPE,LaleyeP,BokoM,vanGestelCA,AhissouH,AkponaS,vanHattumB,SwartK,vanStraalenNM.2006.ContaminationoffishbyorganochlorinepesticideresiduesintheOuemeRivercatchmentintheRepublicofBenin[J].EnvironInt,(inpress)
- ZhangG,ParkerA,HouseA,MaiB,LiX,KangY,WangZ.2002.SedimentaryrecordsofDDTandHCHinthePearlRiverDelta,SouthChina[J].EnvironSciTechnol,36(17):3671-3677
- ZhaoL,MaYJ,ZhouXH.2002.Effectoforganochlorinepesticideresiduesonagriculturalproductsquality[J].ChineseJournalofEco-Agricultrure,10(3):126-128(inChinese)
- ZhouHY,WongMH.2004.ScreeningoforganochlorinesinfreshwaterfishcollectedfromthePearlRiverDelta,People’sRepublicofChina[J].ArchEnvironContamToxicol,46(1):106-113
- ZhouJL,MaskaouiK,QiuYW,HongHS,WangZD.2001.PolychlorinatedbiphenylcongenersandorganochlorineinsecticidesinthewatercolumnandsedimentsofDayaBay,China[J].EnvironPollut,113(3):373-384
- 安太成,陈嘉鑫,傅家谟,盛国英,李桂英,胡振宇,匡耀求.2005.珠三角地区POPs农药的污染现状及控制对策[J].生态环境,14:981-986
- 李卫华,张蕴晖,范奇元,NakataH,KitanoT,AbeS,丁训成.2005.上海和宜兴地区食品和人乳组织中有机氯农药污染现状[J].环境与职业医学,22:14-16
- 梁春穗,邓峰,黄伟雄,李海,陈明,刘子文,染旭霞,梁富荣,蔡文华,梁红洁.2003.广东省食物中化学污染物的网点监测与动态分析[J].中国食品卫生杂志,15:395-401
- 罗孝俊,陈社军,麦碧娴,曾永平.2006.珠江三角洲地区水体表层沉积物中多环芳烃的来源、迁移及生态风险评价[J].生态毒理学报,1(1):17-24
- 王茂起,王竹天,冉陆,韩宏伟,王永芳,杨大进.2003.2000-2001年中国食品污染物监测研究[J].卫生研究,32:322-326
- 吴湘生.2006.中国渔业产业区域竞争力分析与未来发展战略[OL].2006-5-10.http://www.chinafeed.org.cn/cms/_code/business/include/php/180687.htm
- 赵玲,马永军,周旭辉.2002.有机氯农药残留对农产品质量的影响分析[J].中国生态农业学报,10:126-128